无介体MFC微生物催化剂的“独立驯化”与“在线驯化”结合研究

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无介体MFC微生物催化剂的“独立驯化”与“在线驯化”结合研究

化学工程 | 更新时间：2023-11-14

- 无介体MFC微生物催化剂的“独立驯化”与“在线驯化”结合研究
- Research on “independent” and“on-line” acclimation of bacteria catalyzer in microbial fuel cell
- 工程科学与技术 2011年43卷第1期页码：201-207
- 作者机构：
  
  四川大学建筑与环境学院
- 作者简介：
- 基金信息：
  
  四川省科技厅应用基础研究项目（2008JY0042）
- DOI：
  中图分类号：
- 纸质出版日期：2011，
  
  网络出版日期：2009-11-29，
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谢晴.无介体MFC微生物催化剂的“独立驯化”与“在线驯化”结合研究[J].工程科学与技术,2011,43(1):201-207.

Xie Qing. Research on “independent” and“on-line” acclimation of bacteria catalyzer in microbial fuel cell[J]. Advanced Engineering Sciences, 2011,43(1):201-207.
谢晴.无介体MFC微生物催化剂的“独立驯化”与“在线驯化”结合研究[J].工程科学与技术,2011,43(1):201-207. DOI：

Xie Qing. Research on “independent” and“on-line” acclimation of bacteria catalyzer in microbial fuel cell[J]. Advanced Engineering Sciences, 2011,43(1):201-207. DOI：

摘要

中文摘要: 摘要：采用独立驯化和在线驯化相结合的新颖方式，以碳毡、碳布和碳纸为阳极挂膜材料，考察驯化方式和阳极材料对无介体微生物燃料电池（MFC）产电性能和有机物去除效果的影响。结果表明，独立驯化期阳极材料特性对微生物挂膜的影响较大，扫描电镜结果表明挂膜效果最好的是碳毡，碳布次之，碳纸较差；在线驯化约10h后，微生物催化剂的电化学活性显著升高，第2个周期电压达到峰值(碳毡、碳布、碳纸，峰电压分别为0.803V，0.604V和0.574V)，第3个周期MFC能长时间稳定运行。其中碳毡MFC电压平台维持在0.78V左右长达180h；比较MFCs的产电能力优劣顺序为：碳毡(1339.6 mW/m3)＞碳纸(96.8mW/m3) ＞碳布(80mW/m3)，COD去除率为：碳毡(89.5%)＞碳纸(79%)＞碳布(74.7%)。该法无须刮移生物膜

操作简便，阳极产电性能高于文献报道，利于推广。

Abstract

Abstract:Abstract：A novel acclimation of “independent”and “on-line” was developed to study the power generation performance of this acclimate mode with three anodic materials including carbon felt

carbon cloth and carbon paper. The experimental results showed that the anodic characters such as the surface area

aperture distribution

surface roughness and surface electric potential had directly affected the biomass on anode in the period of “independent acclimation”. It was clear that the anodic materials were in turn carbon felt

carbon cloth and carbon paper for abundant biomass on it by SEM. After about 10h in “on-line acclimation”

the electrocatalytic activity of bacteria catalyzer was increased significantly. In the second cycle

the output voltages for MFCs reached the peak (carbon felt/0.803V; carbon cloth/0.604V; carbon paper/0.574V). In the third cycle

MFCs maintained a high stable running for long period

especially the carbon felt-biofilm，the maximal output voltage (0.78V) of it could keep more than 180h. Comparing with power density of MFCs

the priority was in turn the carbon felt (1339.6 mW/m3)

carbon paper (96.8mW/m3) and carbon cloth (80mW/m3). The efficiencies of COD removal were in turn carbon felt (89.5%)

carbon paper (79%) and carbon cloth (74.7%). The main merits of the acclimation were convenient operations and high electrical functions.

关键词

微生物燃料电池(MFC)驯化生物膜产电细菌

Keywords

Microbial fuel cell (MFC)AcclimationBiofilmElectro-microorganism

references

Cristian Picioreanu ；Ian M. Head ；Krishna P. Katuri ；Mark C.M. van Loosdrecht ；Keith Scott,A computational model for biofilm-based microbial fuel cells,Water Research ,2007, 41(13).

Hong Liu ；Bruce E.Logan,Electricity Generation Using an Air-Cathode Single Chamber Microbial Fuel Cell in the Presence and Absence of a Proton Exchange Membrane,Environmental Science & Technology ,2004, 38(14).

SHAOAN CHENG ；HONG LIU ；BRUCE E.LOGAN,Increased Power Generation in a Continuous Flow MFC with Advective Flow through the Porous Anode and Reduced Electrode Spacing,Environmental Science & Technology ,2006, 40(7).

Rabaey, K ；Boon, N ；Siciliano, SD ；Verhaege, M ；Verstraete, W,Biofuel cells select for microbial consortia that self-mediate electron transfer,Applied and Environmental Microbiology ,2004, 70(9).

Juliane N;Uwe S;Miriam R,Fluorinated polyanilines as superior materials for electrocatalytic anodes in bacterial fuel cells,Electrochemistry Communications,2004.

He, Z ；Minteer, SD ；Angenent, LT,Electricity generation from artificial wastewater using an upflow microbial fuel cell,Environmental Science & Technology ,2005, 39(14).

R.Cresson ；H.Carrere ；J.P.Delgenes ；N.Bernet,Biofilm formation during the start-up period of an anaerobic biofilm reactor-Impact of nutrient complementation,Biochemical Engineering Journal ,2006, 30(1).

连静,冯雅丽,李浩然.直接微生物燃料电池的构建及初步研究[J].过程工程学报,2006(3)

Lovley DR,Microbial fuel cells: novel microbial physiologies and engineering approaches.,Current Opinion in Biotechnology ,2006, 17(3).

国家环境保护总局,水和废水监测分析方法,北京:中国环境科学出版社,2002.

KORNEEL RABAEY ；NICO BOON ；MONICA HOFTE ；WILLY VERSTRAETE,Microbial Phenazine Production Enhances Electron Transfer in Biofuel Cells,Environmental Science & Technology ,2005, 39(9).

Cho, EJ ；Ellington, AD,Optimization of the biological component of a bioelectrochemical cell,Bioelectrochemistry ,2007, 70(1).

Finkelstein, DA ；Tender, LM ；Zeikus, JG,Effect of electrode potential on electrode-reducing microbiota,Environmental Science & Technology ,2006, 40(22).

Booki Min ；Bruce E.Logan,Continuous Electricity Generation from Domestic Wastewater and Organic Substrates in a Flat Plate Microbial Fuel Cell,Environmental Science & Technology ,2004, 38(21).

Hong Liu ；Ramanathan Ramnarayanan ；Bruce E.Logan,Production of Electricity during Wastewater Treatment Using a Single Chamber Microbial Fuel Cell,Environmental Science & Technology ,2004, 38(7).

Daniel R. Bond ；Derek R. Lovley,Electricity Production by Geobacter sulfurreducens Attached to Electrodes,Applied and Environmental Microbiology ,2003, 69(3).

易丹,陶虎春,李兆飞.双室微生物燃料电池利用乙酸钠和淀粉产电研究[J].环境科学研究,2008(3)

叶晔捷,宋天顺,徐源.用高浓度对苯二甲酸溶液产电的微生物燃料电池[J].环境科学,2009(4)

卢娜;周顺桂;倪晋仁.微生物燃料电池的产电机制[J].化学进展,2008(7/8)

黄霞;范明志;梁鹏.微生物燃料电池阳极特性对产电性能的影响[J].中国给水排水,2007(3)

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